Identifying the mechanical properties and surface morphology of artocarpus elasticus fiber biocomposites due to the effect of alkali treatment for automotive applications

Authors

DOI:

https://doi.org/10.15587/1729-4061.2025.337175

Keywords:

Artocarpus elasticus, biocomposites, hand lay-up, mechanical properties, morphology, sodium hydroxide

Abstract

Lantung bark (Artocarpus elasticus), a natural fiber abundant in Bengkulu and other Indonesian regions, was studied as reinforcement in polyester-based biocomposites. The increasing demand for environmentally friendly materials has driven the development of natural fiber-based biocomposites as alternatives to synthetic materials. The main problem addressed is the weak interfacial bonding between untreated Lantung fibers and polymer matrices, reducing composite mechanical performance. To overcome this, fibers were treated with Sodium Hydroxide (NaOH) solutions at 2%, 4%, and 6% concentrations for 2 hours to improve surface morphology and chemical reactivity. After drying, treated fibers were fabricated into biocomposites using the hand lay-up pressing method. Testing included morphological observation via 3D microscopy and mechanical evaluation through tensile and bending tests based on ASTM standards. Results showed that 2% NaOH treatment provided the best biocomposite’s mechanical properties, with a Modulus of Rupture (MOR) of 82.41 MPa and a Modulus of Elasticity (MOE) of 4.71 GPa. These improvements are explained by effective removal of surface impurities without significant fiber damage, enhancing fiber-matrix adhesion. The distinctive feature of this study is identifying an optimal alkali concentration that maintains fiber integrity while significantly improving mechanical performance. The developed Lantung biocomposites have potential applications as eco-friendly interior or non-structural automotive components requiring moderate tensile strength and high flexural performance

Author Biographies

Tri Mulyanto, Gunadarma University

Doctor of Information of Technology, Lecturer

Department of Mechanical Engineering

Firda Aulya Syamani, National Research and Innovation Agency

Doctor, Researcher

Research Centre for Biomass and Bioproducts

Ismadi Ismadi, National Research and Innovation Agency

PhD Candidate, Researcher

Research Centre for Biomass and Bioproducts

Deni Purnomo, National Research and Innovation Agency

PhD Candidate, Researcher

Research Centre for Biomass and Bioproducts

Mona Nurjanah, Gunadarma University

Bachelor of Engineering

Department of Mechanical Engineering

Iman Setyadi, Politeknik Negeri Jakarta

Master of Engineering, Lecturer

Department of Mechanical Engineering

Abdul Azis Abdillah, University of Birmingham; Politeknik Negeri Jakarta

PhD Candidate

CASE Automotive Research Centre

Department of Mechanical Engineering

Lecturer

Department of Mechanical Engineering

Sulaksana Permana, Gunadarma University; Universitas Indonesia

Doctor of Engineering in Metallurgy and Materials, Lecturer

Department of Mechanical Engineering

Department of Metallurgy and Materials

References

  1. Yogesh, M., Hari, R. A. N. (2017). Study on Pineapple Leaves Fibre and its Polymer based Composite: A Review. International Journal of Science and Research (IJSR), 6 (1), 799–807. https://doi.org/10.21275/art20164188
  2. Melyna, E., Afridana, A. P. (2023). The Effect of Coffee Husk Waste Addition with Alkalisation Treatment on the Mechanical Properties of Polypropylene Composites. Equilibrium Journal of Chemical Engineering, 7 (1), 14. https://doi.org/10.20961/equilibrium.v7i1.68556
  3. Zin, M. H., Abdan, K., Mazlan, N., Zainudin, E. S., Liew, K. E. (2018). The effects of alkali treatment on the mechanical and chemical properties of pineapple leaf fibres (PALF) and adhesion to epoxy resin. IOP Conference Series: Materials Science and Engineering, 368, 012035. https://doi.org/10.1088/1757-899x/368/1/012035
  4. Khan, M., Rahamathbaba, S., Mateen, M., Ravi Shankar, D., Manzoor Hussain, M. (2019). Effect of NaOH treatment on mechanical strength of banana/epoxy laminates. Polymers from Renewable Resources, 10 (1-3), 19–26. https://doi.org/10.1177/2041247919863626
  5. Peng, X., Zhong, L., Ren, J., Sun, R. (2010). Laccase and alkali treatments of cellulose fibre: Surface lignin and its influences on fibre surface properties and interfacial behaviour of sisal fibre/phenolic resin composites. Composites Part A: Applied Science and Manufacturing, 41 (12), 1848–1856. https://doi.org/10.1016/j.compositesa.2010.09.004
  6. Gundara, G., Nurzein, A. S., Wagiman, A., Ramadhan, A. R. (2023). Effect of Alkalized Pineapple Leaf Fiber Direction Variations on Tensile Strength and Bending of Polyester Matrix Composites. Formosa Journal of Sustainable Research, 2 (1), 87–96. https://doi.org/10.55927/fjsr.v2i1.2703
  7. Aravindh, M., Sathish, S., Ranga Raj, R., Karthick, A., Mohanavel, V., Patil, P. P. et al. (2022). A Review on the Effect of Various Chemical Treatments on the Mechanical Properties of Renewable Fiber-Reinforced Composites. Advances in Materials Science and Engineering, 2022, 1–24. https://doi.org/10.1155/2022/2009691
  8. Annamalai, K., Soundararajan, S., Kalidas, S., Marialueedass, N. (2024). Explorations into the mechanical properties of composites reinforced with sisal and abaca natural fibers. Matéria (Rio Janeiro). https://doi.org/10.1590/1517-7076-rmat-2024-0585
  9. Kabir, M. M., Alhaik, M. Y., Aldajah, S. H., Lau, K. T., Wang, H., Islam, M. M. (2021). Effect of Hemp Fibre Surface Treatment on the Fibre‐Matrix Interface and the Influence of Cellulose, Hemicellulose, and Lignin Contents on Composite Strength Properties. Advances in Materials Science and Engineering, 2021 (1). https://doi.org/10.1155/2021/9753779
  10. Setswalo, K., Molaletsa, N., Oladijo, O. P., Akinlabi, E. T., Sanjay, M. R., Siengchin, S. (2021). The Influence of Fiber Processing and Alkaline Treatment on the Properties of Natural Fiber-reinforced Composites: A Review. Applied Science and Engineering Progress. https://doi.org/10.14416/j.asep.2021.08.005
  11. Torres, G. B., Hiranobe, C. T., da Silva, E. A., Cardim, G. P., Cardim, H. P., Cabrera, F. C. et al. (2023). Eco-Friendly Natural Rubber–Jute Composites for the Footwear Industry. Polymers, 15 (20), 4183. https://doi.org/10.3390/polym15204183
  12. Osman, Z., Elamin, M., Ghorbel, E., Charrier, B. (2025). Influence of Alkaline Treatment and Fiber Morphology on the Mechanical, Physical, and Thermal Properties of Polypropylene and Polylactic Acid Biocomposites Reinforced with Kenaf, Bagasse, Hemp Fibers and Softwood. Polymers, 17 (7), 844. https://doi.org/10.3390/polym17070844
  13. Atmakuri, A., Palevicius, A., Janusas, G., Eimontas, J. (2022). Investigation of Hemp and Flax Fiber-Reinforced EcoPoxy Matrix Biocomposites: Morphological, Mechanical, and Hydrophilic Properties. Polymers, 14 (21), 4530. https://doi.org/10.3390/polym14214530
  14. Hestiawan, H., Zuliantoni, Supardi, N. I., Sudibyo (2025). Characteristics of Lantung Fiber and the Effect of Alkali Treatment and Water Absorption on the Mechanical Properties of Lantung Fiber Reinforced Composites. Jordan Journal of Mechanical and Industrial Engineering, 19 (02), 469–478. https://doi.org/10.59038/jjmie/190217
  15. Abraha, K. G., Debeli, D. K., Ghani, M. U., Tesfahunegn, A. A., Guo, J. (2023). Enset Fiber-Reinforced Polylactic Acid-Based Biocomposites for High-Performance Application. Journal of Composites Science, 7 (10), 407. https://doi.org/10.3390/jcs7100407
  16. Fadhillah, A. R., Hermawan, D., Wardhani, A. R. (2020). Pengaruh prosentase larutan NaOH pada proses alkalisasi serat kulit pohon waru (hibiscus tiliaceus) sebagai reinforcement komposit terhadap kekuatan tarik serat tunggal. Turbo : Jurnal Program Studi Teknik Mesin, 8 (2). https://doi.org/10.24127/trb.v8i2.1159
  17. Karthikeyan, A., Balamurugan, K., Kalpana, A. (2014). The effect of sodium hydroxide treatment and fiber length on the tensile property of coir fiber-reinforced epoxy composites. Science and Engineering of Composite Materials, 21 (3). https://doi.org/10.1515/secm-2013-0130
  18. ASTM D3039/D3039M-17. Test Method for Tensile Properties of Polymer Matrix Composite Materials. https://doi.org/10.1520/d3039_d3039m-17
  19. Saba, N., Paridah, M. T., Abdan, K., Ibrahim, N. A. (2016). Effect of oil palm nano filler on mechanical and morphological properties of kenaf reinforced epoxy composites. Construction and Building Materials, 123, 15–26. https://doi.org/10.1016/j.conbuildmat.2016.06.131
  20. Malalli, C. S., Ramji, B. R. (2022). Mechanical characterization of natural fiber reinforced polymer composites and their application in Prosthesis: A review. Materials Today: Proceedings, 62, 3435–3443. https://doi.org/10.1016/j.matpr.2022.04.276
  21. Firda, M. (2025). Image of The Morphology Test Results of Lantung Bark (Artocarpus Elasticus). Research Center for Biomass and Bioproduct, National Research and Innovation Agency. Available at: https://drive.google.com/file/d/199r4myKg5-j3zEMVN9jDEx1m71-P1_t1/view?usp=drive_link
  22. Firda, M. (2025). Tensile Test Results of Artocarpus Elasticus Fibers Treated with Sodium Hydroxide (NaOH). Research Center for Biomass and Bioproduct, National Research and Innovation Agency. Available at: https://drive.google.com/file/d/1PWZMPA8r4U8qj6fsFwvehHM0RYkz3S6y/view?usp=drive_link
  23. Firda, M. (2025). Bending Test Results of Artocarpus Elasticus Fibers Treated with Sodium Hydroxide (NaOH). Research Center for Biomass and Bioproduct, National Research and Innovation Agency. Available at: https://drive.google.com/file/d/1AmL4tgckzHtOttyHhqFuQXhGf9abBNly/view?usp=drive_link
  24. Fitri, M., Mahzan, S., Anggara, F. (2021). The Mechanical Properties Requirement for Polymer Composite Automotive Parts - A Review. International Journal of Advanced Technology in Mechanical, Mechatronics and Materials, 1 (3), 125–133. https://doi.org/10.37869/ijatec.v1i3.38
  25. Kumar, R. S., Muralidharan, N., Sathyamurthy, R. (2020). Optimization of Alkali Treatment Process Parameters for Kenaf Fiber: Experiments Design. Journal of Natural Fibers, 19 (11), 4276–4285. https://doi.org/10.1080/15440478.2020.1856276
  26. Simamora, P., Simanjuntak, J., Sinulingga, K., Laksono, A. D. (2023). Mechanical Properties of Polypropylene Composites with different Reinforced Natural Fibers – A Comparative Study. Journal of Ecological Engineering, 24 (7), 311–317. https://doi.org/10.12911/22998993/164757
Identifying the mechanical properties and surface morphology of artocarpus elasticus fiber biocomposites due to the effect of alkali treatment for automotive applications

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Published

2025-08-27

How to Cite

Mulyanto, T., Syamani, F. A., Ismadi, I., Purnomo, D., Nurjanah, M., Setyadi, I., Abdillah, A. A., & Permana, S. (2025). Identifying the mechanical properties and surface morphology of artocarpus elasticus fiber biocomposites due to the effect of alkali treatment for automotive applications. Eastern-European Journal of Enterprise Technologies, 4(12 (136), 21–30. https://doi.org/10.15587/1729-4061.2025.337175

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Materials Science